@Article{AlbuquerqueLoFrTaFaNoGa:2005:ImDiRa,
author = "Albuquerque, Leila Maria Merc{\^e} de and Longo, Karla Maria and
Freitas, Saulo Ribeiro de and Tarasova, Tatiana and Fattori, A.
Plana and Nobre, Carlos Afonso and Gatti, L. V.",
affiliation = "Instituto Nacional de Pesquisas Espaciais (INPE); Universidade
Federal de Mato Grosso do Sul, UFMS, DHT, Brazil and {Instituto
Nacional de Pesquisas Espaciais (INPE)} and {Instituto Nacional de
Pesquisas Espaciais (INPE)} and {Instituto Nacional de Pesquisas
Espaciais (INPE)} and Universidade Federal de Mato Grosso do Sul,
UFMS, DHT, Brazil and {Instituto Nacional de Pesquisas Espaciais
(INPE)} and Instituto de Pesquisas Energeticas e Nucleares (IPEN
/USP), Brazil",
title = "Sensitivity studies on the photolysis rates calculation in
Amazonian atmospheric chemistry – Part I: The impact of the direct
radiative effect of biomass burning aerosol particles",
journal = "Atmospheric Chemistry and Physics Discussion",
year = "2005",
volume = "5",
number = "5",
pages = "9325--9353",
month = "Set",
note = "{SRef-ID: 1680-7375/acpd/2005-5-9325}",
abstract = "The impact of the direct radiative effect of the aerosol particles
on the calculation of the photolysis rates and consequently on the
atmospheric chemistry in regional smoke clouds due to biomass
burning over the Amazon basin is addressed in this work. It
explores a case study for 19 September 2002 at LBA-RACCI-SMOCC
(The Large-Scale Biosphere-Atmosphere experiment in Amazonia
Radiation, Cloud, and Climate Interactions Smoke, Aerosols,
Clouds, Rainfall and Climate) pasture site in SW Amazonia. The
Tropospheric Ultraviolet Visible radiation model (TUV) version
4.2, (Madronich et al., 1987) is used for the photolysis rates
calculation considering the layer aerosol optical depth from the
Coupled Aerosol Tracer Transport model to the Brazilian Regional
Atmospheric Modeling System (CATT-BRAMS) (Freitas et al., 2005). A
dynamical aerosol model (Proc{\'o}pio et al., 2003) is included
in the radiative transfer model to take into account the high
temporal variability of the aerosol optical thickness. This
methodology is tested by comparing modeled and measured clear sky
solar irradiances. The results show a good agreement with measured
PAR radiation values. The actinic flux attenuation, for AOT (500
nm) values around 1.94, decreases the photolysis rates by about
70% in the presence of near-ground smoke aerosol and above the
smoke layer the photolysis process tends to increase by about 40%.
A simulation of the ozone production is carried out using a
one-dimensional photochemical box model and comparisons with
observation are shown.",
copyholder = "SID/SCD",
issn = "1680-7375",
language = "en",
targetfile = "Albuquerque_Sensitivity.pdf",
urlaccessdate = "26 abr. 2024"
}